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That work presents a computational read of Rh III -catalyzed amalgamation of 1,2-benzothiazines from NH-sulfoximines and diazo compounds reported by Bolm et al. The reaction entails five sequent processes: Phenyl sulfoximine is found to be the most favorable substrate with the lowest barrier in comparison with methoxybenzene sulfoximine and nitrobenzene sulfoximine.

The noncovalent interaction is indicated to be mainly responsible payment the experimentally observed regioselectivity.

The theoretical results are expected to provide valuable guidance and help for the synthesis of 1,2-benzothiazines.

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